Dephasing in Quantum Dots: Quadratic Coupling to Acoustic Phonons

A microscopic theory of optical transitions in quantum dots with carrier-phonon interaction is developed. Virtual transitions into higher confined states with acoustic phonon assistance add a quadratic phonon coupling to the standard linear one, thus extending the independent Boson model. Summing infinitely many diagrams in the cumulant, a numerically exact solution for the interband polarization is found. Its full time dependence and the absorption lineshape of the quantum dot are calculated. It is the quadratic interaction which gives rise to a temperature-dependent broadening of the zero-phonon line, being here calculated for the first time in a consistent scheme.Comment: 4 pages, 2 figure

Evaluation of the importance of spin-orbit couplings in the nonadiabatic quantum dynamics with quantum fidelity and with its efficient "on-the-fly" ab initio semiclassical approximation

We propose to measure the importance of spin-orbit couplings (SOCs) in the nonadiabatic molecular quantum dynamics rigorously with quantum fidelity. To make the criterion practical, quantum fidelity is estimated efficiently with the multiple-surface dephasing representation (MSDR). The MSDR is a semiclassical method that includes nuclear quantum effects through interference of mixed quantum-classical trajectories without the need for the Hessian of potential energy surfaces. Two variants of the MSDR are studied, in which the nuclei are propagated either with the fewest-switches surface hopping or with the locally mean field dynamics. The fidelity criterion and MSDR are first tested on one-dimensional model systems amenable to numerically exact quantum dynamics. Then, the MSDR is combined with "on-the-fly" computed electronic structure to measure the importance of SOCs and nonadiabatic couplings (NACs) in the photoisomerization dynamics of CH2NH2+ considering 20 electronic states and in the collision of F + H2 considering six electronic states.Comment: 9 pages, 3 figures, submitted to J. Chem. Phy

Spatially resolved photo ionization of ultracold atoms on an atom chip

We report on photo ionization of ultracold magnetically trapped Rb atoms on an atom chip. The atoms are trapped at 5 $\mu$K in a strongly anisotropic trap. Through a hole in the chip with a diameter of 150 $\mu$m two laser beams are focussed onto a fraction of the atomic cloud. A first laser beam with a wavelength of 778 nm excites the atoms via a two photon transition to the 5D level. With a fiber laser at 1080 nm the excited atoms are photo ionized. Ionization leads to depletion of the atomic density distribution observed by absorption imaging. The resonant ionization spectrum is reported. The setup used in this experiment is not only suitable to investigate BEC ion mixtures but also single atom detection on an atom chip

High-temperature ferroelectric order and magnetic field-cooled effect driven magnetoelectric coupling in R2BaCuO5 (R= Er, Dy, Sm)

The high-temperature ferroelectric order and a remarkable magnetoelectric effect driven by the magnetic field cooling are reported in R2BaCuO5 (R = Er, Dy, Sm) series. The ferroelectric (FE) orders are observed at much higher temperatures than their magnetic orders for all three members. The value of FE Curie temperature (TFE) is considerably high as ~ 235 K with the polarization value (P) of ~ 1410 {\mu}C/m2 for a 4 kV/cm poling field in case of Er2BaCuO5, whereas the values of TFE and P are also promising as ~ 232 K and ~ 992 {\mu}C/m2 for Dy2BaCuO5, and ~ 184 K and ~ 980 {\mu}C/m2 for Sm2BaCuO5. The synchrotron diffraction studies of Dy2BaCuO5 confirm a structural transition at TFE to a polar Pna21 structure, which correlates the FE order. An unusual magnetoelectric coupling is observed below the R order for Er and Dy compounds and below the Cu order for Sm compound, when the pyroelectric current is recorded only with the magnetic field both in heating and cooling cycles i.e. typical magnetic field cooled effect. The magnetic field cooled effect driven emergence of polarization is ferroelectric in nature, as it reverses due to the opposite poling field. The unexplored R2BaCuO5 series attracts the community for large TFE, high P value, and strange magnetoelectric consequences.Comment: 9 figures and 2 supporting figure